Successful prediction of pathways of storm runoff generation and associated soil erosion is of considerable societal importance, including off-site impacts such as water quality and the provision of related ecosystem services. Recently, the role of connectivity in controlling runoff and erosion has received significant and increasing scientific attention, though in a disparate and uncoordinated way. There is a wealth of experience and expertise in connectivity across Europe that could be harnessed to ensure that the potential already demonstrated in key studies can be more widely fulfilled; to move forward along agreed lines and identify emerging goals, and to benefit from cross-fertilization of ideas from the fields of Hydrology, Soil Science, Geomorphology and Ecology.